Roushan
@roushanpsingh
Grad student @ChemistryatUIC alumnus @iiserbhopal
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Excited to share our new article which explores coordination-induced O-H and N-H bond weakening using earth-abundant metals like aluminum and iron! Did you know weakening these bonds is crucial for targeted reactivity and renewable energy? Thank you @NealMankad @SoumenSinha87
I'm pleased to share our first publication in @NatureComms led by @SoumenSinha87 @roushanpsingh. A pleasure to collaborate with Dan Ess & team again! doi.org/10.1038/s41467…
Thanks to Dan Ess for bringing us along for the ride on this one @roushanpsingh pubs.acs.org/doi/10.1021/ac…
pubs.acs.org
CpFe(CO)2 Radical Generated from Dinuclear [CpFe(CO)2]2 and Mononuclear (Cp)(CO)2Fe(H): Density...
Density functional theory (DFT) methods remain the most practical approach to calculating properties and reaction mechanisms of transition metal complexes. While the accuracy of DFT methods has been...
Can AI accelerate reaction discovery in photocatalysis? We (@GloriusGroup) present a data-driven strategy to unlock the triplet-state reactivity of monocyclic heteroarenes, enabling EnT-catalyzed intermolecular dearomative cycloadditions. Now in @J_A_C_S! pubs.acs.org/doi/10.1021/ja…
pubs.acs.org
Accelerated Discovery of Energy Transfer-Catalyzed Dearomative Cycloadditions through a Data-Driven...
Visible-light-mediated energy transfer (EnT) photocatalysis has emerged as a highly appealing strategy for converting planar (hetero)arenes into complex, medicinally relevant, three-dimensional (3D)...
Excited to share our group's strategies to stabilize mononuclear Al radicals! Redox-active ligands + strained geometries give Al biphilic character, letting it mimic d-/f-block metals. Thanks @NealMankad for the guidance!
Check out our Perspective on Al(II) chemistry in @JACS_Au led by @roushanpsingh. Thanks to the editors for inviting us to participate in their special issue on sustainable small molecule activation! doi.org/10.1021/jacsau…
We are excited to announce our @J_A_C_S paper on frameworks with metalloprotein-like sites! ɑ-helices designed to assemble by metal-coordination and the hydrophobic effect. Point mutations yield unique frameworks with diverse metalloprotein-like sites. tinyurl.com/jk62cb27
🚨 New in @J_A_C_S : The @GlusacGroup at @UIC has developed a new MOF composed of nanographene ligands (hexa-peri-hexabenzocoronene), which acts as a photocatalyst for CO2 reduction using water as the terminal electron donor. Read it here! pubs.acs.org/doi/10.1021/ja…
Our publication in @J_A_C_S demonstrates that aluminum radicals can reduce carbon dioxide (CO2) through a single electron reduction which is typically thermodynamically less favorable. I am grateful to my PI, @NealMankad, for his constant support and motivation.
Our latest Al-Fe research is published in @J_A_C_S. Led by my student Roushan @ChemistryatUIC and our collaboration with Dan Ess of BYU, we are starting to map the chemistry of Al(II) through this mild approach! doi.org/10.1021/jacs.5…
📣 Research from the lab of @andy_i_nguyen makes the cover for the newest issue of @ChemEurJ! The work uncovered previously elusive metallopeptide structures that could enable new bioinorganic chemistry. Read the article: bit.ly/4fkHnRD
What a week! The AIMED Workshop on Heterogeneous Catalysis was a remarkable success after nearly a year of prep. We couldn't have picked a better time - the excitement is at an all-time high, with two Nobel Prizes recognizing AI and fueling the momentum for scientific discovery!
The LdippAl(Me) radical exhibits reactivity comparable to divalent F-block elements. A comprehensive analysis of heterobimetallic electronic structures demonstrates the mechanistic diversity that arises from systems combining p-block and d-block metals. Thank you @NealMankad!
Fresh off presenting the work at CRIC-5 this weekend, check out the latest study by @roushanpsingh on Al/M chemistry published in @InorgChem doi.org/10.1021/acs.in…
pubs.acs.org
Frustrated Al/M Heterobimetallic Complexes (M = Cr, Mo, W) That Exhibit Both Lewis and Radical Pair...
Exploration of new heterobinuclear Al/M combinations is relevant to contemporary strategies for cooperative bond activation. Here, we report the synthesis and characterization of six new Al/M...
And that’s a wrap for CRIC-5! > 100 attendees, 50+ poster contributions and 22 talks. Midwest is best 😎
Clock is ticking! 🕒 Tomorrow's FREE #ACSScienceTalks event with @iiserbhopal's Manmohan Kapur will showcase how to functionalize C-H bonds distally via the prcoess of Electrophilic C-H Metallation. Register now: brnw.ch/21wK3kV #ACSInternational #Chemistry
Second installment from my "PI is back in the lab" phase a couple years ago is out in @Orgmet_ACS. Thanks to @SollogoubM for the trans-Atlantic collaboration!
Supramolecular Perturbation of Metal–Metal Bonding in Cyclodextrin-Encapsulated (NHC)Cu-FeCp(CO)2 Complexes. New in @Orgmet_ACS from @NealMankad and colleagues. Please have a look: pubs.acs.org/doi/10.1021/ac…
I'm pleased to share our first publication in @NatureComms led by @SoumenSinha87 @roushanpsingh. A pleasure to collaborate with Dan Ess & team again! doi.org/10.1038/s41467…
A couple years ago during a less busy phase, I thought it would be fun to work in the lab again. One of the products from that period is now published @ChemicalScience! I have always wanted to achieve a single-author paper! doi.org/10.1039/D3SC05…
I am excited to share a perspective in ACS Catalysis on molecular Al/M heterobimetallic catalysis. Thank you @NealMankad and @SoumenSinha87 pubs.acs.org/doi/10.1021/ac…
Congratulations to my co-workers @roushanpsingh and @SoumenSinha87 for publishing a nice Perspective in @ACSCatalysis on molecular Al/M heterobimetallic catalysis: doi.org/10.1021/acscat…
Congratulations to my co-workers @roushanpsingh and @SoumenSinha87 for publishing a nice Perspective in @ACSCatalysis on molecular Al/M heterobimetallic catalysis: doi.org/10.1021/acscat…
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